Article
Electron Emission in the Near-Field of Surface Plasmons
Surface Science
(2013)
Abstract
Plasmon-enhanced photoelectron emission in the near-field region of gold nanostructures is reported. We show that, depending on the photon energy of the excitation light, the emission from the near-field region can be markedly stronger than from the plasmonic gold itself. Photoemission micrographs also indicate that the spatial confinement of the near-field emission is stronger than in the gold and that the near-field emission exhibits a strong sensitivity on the linear and circular polarization state of the excitation light. The results are explained in terms of work-function differences between the near-field region and the plasmonic material and an interaction between propagating and localized surface plasmon modes. We suggest that the circular polarization sensitivity of the near-field surface plasmon modes may open the way to generate spin-polarized electrons in a plasmon-induced photoemission process.
Disciplines
Publication Date
January, 2013
DOI
10.1016/j.susc.2012.08.026
Publisher Statement
Plasmon-enhanced photoelectron emission in the near-field region of gold nanostructures is reported. We show that, depending on the photon energy of the excitation light, the emission from the near-field region can be markedly stronger than from the plasmonic gold itself. Photoemission micrographs also indicate that the spatial confinement of the near-field emission is stronger than in the gold and that the near-field emission exhibits a strong sensitivity on the linear and circular polarization state of the excitation light. The results are explained in terms of work-function differences between the near-field region and the plasmonic material and an interaction between propagating and localized surface plasmon modes. We suggest that the circular polarization sensitivity of the near-field surface plasmon modes may open the way to generate spin-polarized electrons in a plasmon-induced photoemission process.
Citation Information
Robert Campbell Word, Joseph P.S. Fitzgerald and Rolf Kӧnenkamp. "Electron Emission in the Near-Field of Surface Plasmons" Surface Science Vol. 607 (2013) p. 148 - 152 Available at: http://works.bepress.com/rolf_koenenkamp/20/