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Article
Ultrafast measurement of two-photon absorption by loss modulation
Optics Letters (2002)
  • Peifang Tian, John Carroll University
  • Warren S. Warren
Abstract
We demonstrate a direct and sensitive technique for measuring two-photon absorption (TPA).An intensity- modulated femtosecond laser beam passes through a sample exhibiting TPA.A TPA signal at twice the modulation frequency is then generated and subsequently measured by a lock-in amplifier. The absolute TPA cross section of Rhodamine 6G at 800nm is found to be 15.32.010 -50 cm 4 s / photon and agrees well with previously published results obtained with much higher intensity [J.Chem.Phys. 112, 9201 (2000)]. Our method may be especially useful in measuring nonlinear absorptions of nonfluorescent materials.
Publication Date
September, 2002
Publisher Statement
© 2002 Optical Society of America DOI: 10.1364/OL.27.001634
Citation Information
Peifang Tian and Warren S. Warren. "Ultrafast measurement of two-photon absorption by loss modulation" Optics Letters Vol. 27 Iss. 18 (2002)
Available at: http://works.bepress.com/peifang_tian/8/