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Phase transition in bulk single crystals and thin films of VO2 by nanoscale infrared spectroscopy and imaging
Physical Review B
  • Mengkun Liu, University of California, San Diego
  • Aaron J. Sternbach, University of California, San Diego
  • Martin Wagner, University of California, San Diego
  • Tetiana V. Slusar, Electronics and Telecommunications Research Institute
  • Sergey L. Bud'ko, Iowa State University
  • Salinporn Kittiwatanakul, University of Virginia
  • M. M. Qazilbash, College of William and Mary
  • Alexander McLeod, University of California, San Diego
  • Zhe Fei, University of California, San Diego
  • Elsa Abreu, Boston University
  • Jingdi Zhang, University of California, San Diego
  • Michael Goldflam, University of California, San Diego
  • Siyuan Dai, University of California, San Diego
  • Guang-Xin Ni, University of California, San Diego
  • Jiwei Lu, University of Virginia
  • Hans A. Bechtel, Lawrence Berkeley National Laboratory
  • Michael C. Martin, Lawrence Berkeley National Laboratory
  • Markus B. Raschke, University of Colorado Boulder
  • Richard D. Averitt, University of California, San Diego
  • Stuart A. Wolf, University of Virginia
  • Hyun-Tak Kim, Electronics and Telecommunications Research Institute
  • Paul C. Canfield, Iowa State University
  • D. N. Basov, University of California, San Diego
Document Type
Article
Publication Version
Published Version
Publication Date
6-15-2015
DOI
10.1103/PhysRevB.91.245155
Abstract

We have systematically studied a variety of vanadium dioxide (VO2) crystalline forms, including bulk single crystals and oriented thin films, using infrared (IR) near-field spectroscopic imaging techniques. By measuring the IR spectroscopic responses of electrons and phonons in VO2 with sub-grain-size spatial resolution (∼20nm), we show that epitaxial strain in VO2 thin films not only triggers spontaneous local phase separations, but also leads to intermediate electronic and lattice states that are intrinsically different from those found in bulk. Generalized rules of strain- and symmetry-dependent mesoscopic phase inhomogeneity are also discussed. These results set the stage for a comprehensive understanding of complex energy landscapes that may not be readily determined by macroscopic approaches.

Comments

This article was published in Physical Review B 91 (2015): 245155, doi:10.1103/PhysRevB.91.245155. Posted with permission

Copyright Owner
American Physical Society
Language
en
File Format
application/pdf
Citation Information
Mengkun Liu, Aaron J. Sternbach, Martin Wagner, Tetiana V. Slusar, et al.. "Phase transition in bulk single crystals and thin films of VO2 by nanoscale infrared spectroscopy and imaging" Physical Review B Vol. 91 Iss. 24 (2015) p. 245155
Available at: http://works.bepress.com/paul_canfield/95/