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Article
Nonequilibrium Pair Breaking in Ba(Fe1-xCox)(2)As-2 Superconductors: Evidence for Formation of a Photoinduced Excitonic State
Ames Laboratory Accepted Manuscripts
  • Xu Yang, Iowa State University and Ames Laboratory
  • Liang Luo, Iowa State University and Ames Laboratory
  • M. Mootz, University of Alabama at Birmingham
  • Aaron Patz, Iowa State University and Ames Laboratory
  • Sergey L. Bud’ko, Iowa State University and Ames Laboratory
  • Paul C. Canfield, Iowa State University and Ames Laboratory
  • I. E. Perakis, University of Alabama at Birmingham
  • Jigang Wang, Iowa State University and Ames Laboratory
Publication Date
12-26-2018
Department
Ames Laboratory; Physics and Astronomy
OSTI ID+
1492059
Report Number
IS-J 9790
DOI
10.1103/PhysRevLett.121.267001
Journal Title
Physical Review Letters
Abstract

Ultrafast terahertz (THz) pump-probe spectroscopy reveals an unusual out-of-equilibrium Cooper pair nonlinear dynamics and a nonequilibrium state driven by femtosecond (fs) photoexcitation of superconductivity (SC) in iron pnictides. Following fast SC quench via hot-phonon scattering, a second, abnormally slow (many hundreds of picoseconds), SC quench regime is observed prior to any recovery. Importantly, a nonlinear pump fluence dependence is identified for this remarkably long prebottleneck dynamics that are sensitive to both doping and temperature. Using quantum kinetic modeling we argue that the buildup of excitonic interpocket correlation between electron-hole ( e − h ) quasiparticles (QP) quenches SC after fs photoexcitation leading to a long-lived, many-QP excitonic state.

DOE Contract Number(s)
W911NF-15-1-0135; SC0019137; AC02-07CH11358
Language
en
Publisher
Iowa State University Digital Repository, Ames IA (United States)
Citation Information
Xu Yang, Liang Luo, M. Mootz, Aaron Patz, et al.. "Nonequilibrium Pair Breaking in Ba(Fe1-xCox)(2)As-2 Superconductors: Evidence for Formation of a Photoinduced Excitonic State" Vol. 121 Iss. 26 (2018) p. 267001
Available at: http://works.bepress.com/paul_canfield/169/