Article
Direct 17O Dynamic Nuclear Polarization of Single-Site Heterogeneous Catalysts
Chemical Communications
Document Type
Article
Disciplines
Publication Version
Accepted Manuscript
Publication Date
1-1-2018
DOI
10.1039/C8CC00293B
Abstract
We utilize direct 17O DNP for the characterization of non-protonated oxygens in heterogeneous catalysts. The optimal sample preparation and population transfer approach for 17O direct DNP experiments performed on silica surfaces are determined and applied to the characterization of Zr- and Y-based mesoporous silica-supported single-site catalysts.
Copyright Owner
The Royal Society of Chemistry
Copyright Date
2018
Language
en
File Format
application/pdf
Citation Information
Frederic A. Perras, Kasuni Chathurika Boteju, Igor Ivan Slowing, Aaron D. Sadow, et al.. "Direct 17O Dynamic Nuclear Polarization of Single-Site Heterogeneous Catalysts" Chemical Communications Vol. 54 (2018) p. 3472 - 3475 Available at: http://works.bepress.com/aaron_sadow/54/
This is article is published as Perras, Frédéric A., Kasuni Chathurika Boteju, Igor Ivan Slowing, Aaron D. Sadow, and Marek Pruski. "Direct 17 O Dynamic Nuclear Polarization of Single-Site Heterogeneous Catalysts." Chemical Communications 54 (2018): 3472-3475. DOI: 10.1039/C8CC00293B. Posted with permission.