In a previous paper, the gas-phase acidities of XHn compounds (X= C, N, 0, F, Si, P, S, Cl) were predicted with ab initio wave functions. At the MP4 level of theory with extended basis sets (6-311++G(3df,2pd)3 for second-period atoms and 6-3l++G- (3df,2pd) for third-period atoms], the calculated gas-phase acidities for these species were determined to be within 2 kcaljmol of experimental values. Similar results for the second period were obtained by DeFrees and McLean.