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Presentation
Modeling Free-Carrier Absorption and Avalanching by Ultrashort Laser Pulses
SPIE Laser-Induced Damage in Optical Materials (2011)
  • Jeremy R. Gulley, Kennesaw State University
Abstract

In the past decade it was demonstrated experimentally that negatively-chirped laser pulses can lower the surface LIDT for wide band-gap materials by decreasing the number of photons required for photoionization on the leading edge of the pulse. Similarly, simulations have shown that positively-chirped pulses resulting from selffocusing and self-phase modulation in bulk dielectrics can alter the onset of laser-induced material modifications by increasing the number of photons required for photoionization on the leading edge of the pulse. However, the role of multi-chromatic effects in free-carrier absorption and avalanching has yet to be addressed. In this work a frequency-selective model of free-carrier dynamics is presented, based on a recently extended multi-rate equation for the distribution of electrons in the conduction band. In this model free-carriers gain energy from the field by single-photon absorption at the instantaneous frequency, which varies as a function of space and time. For cases of super-continuum generation it is shown that a Drude-type absorption can vary from 50% to over 200% the absorption rate as evaluated at the central pulse frequency only. Simulations applying this model to ultrafast laser-plasma interactions in fused silica explore how pulse chirps may be used as a distinguishing parameter for LID resulting from otherwise identical pulses.

Keywords
  • Absorption,
  • Dielectrics,
  • Electrons,
  • Laser induced damage,
  • Lasers,
  • Modeling,
  • Modulation,
  • Photons,
  • Plasma,
  • Silica
Publication Date
September, 2011
Citation Information
Jeremy R. Gulley. "Modeling Free-Carrier Absorption and Avalanching by Ultrashort Laser Pulses" SPIE Laser-Induced Damage in Optical Materials (2011)
Available at: http://works.bepress.com/jeremy_gulley/5/