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Overview of the 2010 Carbonaceous Aerosols and Radiative Effects Study (CARES)
Atmospheric Chemistry and Physics
  • Rahul A. Zaveri, Pacific Northwest National Laboratory
  • William J. Shaw, Pacific Northwest National Laboratory
  • Daniel J. Cziczo, Massachusetts Institute of Technology
  • Beat Schmid, Pacific Northwest National Laboratory
  • Richard Ferrare, NASA Langley Research Center
  • M. Lizabeth Alexander, Pacific Northwest National Laboratory
  • Raul Alvarez, NOAA Earth System Research Laboratory
  • W. Patrick Arnott, Desert Research Institute
  • Dean B. Atkinson, Portland State University
  • Sunil Baidar, University of Colorado Boulder
  • Robert M. Banta, NOAA Earth System Research Laboratory
  • James Barnard, Pacific Northwest National Laboratory
  • Josef Beranek, Pacific Northwest National Laboratory
  • Larry K. Berg, Pacific Northwest National Laboratory
  • Fred Brechtel, Brechtel Manufactoring, Inc.
  • W. Alan Brewer, NOAA Earth System Research Laboratory
  • John F. Cahill, University of California - San Diego
  • Brian Cairns, NASA Goddard Institute for Space Studies
  • Christopher D. Cappa, University of California - Davis
  • D. Chand, Pacific Northwest National Laboratory
  • S. China, Los Alamos National Laboratory
  • Jennifer M. Comstock, Pacific Northwest National Laboratory
  • Manvendra K. Dubey, Los Alamos National Laboratory
  • Robert C. Easter, Pacific Northwest National Laboratory
  • M. H. Erickson, Washington State University
  • Jerome Fast, Pacific Northwest National Laboratory
  • Cody Floerchinger, Montana State University - Bozeman
  • B. Flowers, Los Alamos National Laboratory
  • Edward C. Fortner, Aerodyne Research, Inc.
  • Jeffrey S. Gaffney, University of Arkansas - Main Campus
  • Mary K. Gilles, Lawrence Berkeley National Laboratory
  • Kyle Gorkowski, Carnegie Mellon University
  • William Gustafson, Pacific Northwest National Laboratory
  • Madhu Gyawali, University of Nevada - Reno
  • J. Hair, University of Nevada - Reno
  • R. M. Hardesty, NOAA Earth System Research Laboratory
  • Joseph Harworth, Portland State University
  • Scott C. Herndon, Aerodyne Research, Inc.
  • Naruki Hiranuma, Pacific Northwest National Laboratory
  • Chris Hostetler, NASA Langley Research Center
  • John M. Hubbe, Pacific Northwest National Laboratory
  • John T. Jayne, Aerodyne Research, Inc
  • H. Jeong, University of North Dakota
  • B. Tom Jobson, Washington State University
  • Evgueni Kassianov, Pacific Northwest National Laboratory
  • Lawrence I. Kleinman, Brookhaven National Laboratory
  • C. Kluzek, Pacific Northwest National Laboratory
  • W. Berk Knighton, Montana State University - Bozeman
  • Katheryn R. Kolesar, University of California - Davis
  • Chongai Kuang, Brookhaven National Laboratory
  • Alena Kubátová, University of North Dakota
  • Andrew O. Langford, NOAA Earth System Research Laboratory
  • Alexander Laskin, Pacific Northwest National Laboratory
  • N. Laulainen, Pacific Northwest National Laboratory
  • Richard D. Marchbanks, NOAA Earth System Research Laboratory
  • Claudio Mazzoleni, Michigan Technological University
  • Fan Mei, Brookhaven National Laboratory
  • Ryan C. Moffet, University of the Pacific
  • Dan Nelson, Pacific Northwest National Laboratory
  • Michael Obland, NASA Langley Research Center
  • Hilke Oetjen, University of Colorado Boulder
  • Timothy B. Onasch, Aerodyne Research, Inc
  • I. Ortega, University of Colorado Boulder
  • Matteo Ottaviani, NASA Goddard Institute for Space Studies
  • Mikhail Pekour, Pacific Northwest National Laboratory
  • Kimberly A. Prather, University of California - San Diego
  • James Gregory Radney, Portland State University
  • Raymond R. Rogers, NASA Langley Research Center
  • Scott P. Sandberg, NOAA Earth System Research Laboratory
  • Arthur J. Sedlacek, Brookhaven National Laboratory
  • Christoph J. Senff, NOAA Earth System Research Laboratory
  • Gunnar I. Senum, Brookhaven National Laboratory
  • Ari Setyan, University of California - Davis
  • John E. Shilling, Pacific Northwest National Laboratory
  • ManishKumar Shrivastava, Pacific Northwest National Laboratory
  • C. Song, Pacific Northwest National Laboratory
  • Stephen R. Springston, Brookhaven National Laboratory
  • R. Subramanian, Droplet Measurements Technologies
  • Kaitlyn Suski, University of California - San Diego
  • Jason Tomlinson, Pacific Northwest National Laboratory
  • Rainer M. Volkamer, University of Colorado Boulder
  • H. W. Wallace, Washington State University
  • Jian Wang, Brookhaven National Laboratory
  • A. M. Weickmann, NOAA Earth System Research Laboratory
  • Douglas R. Worsnop, Aerodyne Research, Inc.
  • Xiao-Ying Yu, Pacific Northwest National Laboratory
  • Alla Zelenyuk, Pacific Northwest National Laboratory
  • Qi Zhang, University of California - Davis
Document Type
Article
Publication Date
1-1-2012
Subjects
  • Atmospheric aerosols -- Composition -- Analysis,
  • Atmospheric aerosols -- Spectra -- Measurement,
  • Air -- Pollution,
  • Carbon -- Environmental aspects
Abstract

Substantial uncertainties still exist in the scientific understanding of the possible interactions between urban and natural (biogenic) emissions in the production and transformation of atmospheric aerosol and the resulting impact on climate change. The US Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) program’s Carbonaceous Aerosol and Radiative Effects Study (CARES) carried out in June 2010 in Central Valley, California, was a comprehensive effort designed to improve this understanding. The primary objective of the field study was to investigate the evolution of secondary organic and black carbon aerosols and their climate-related properties in the Sacramento urban plume as it was routinely transported into the forested Sierra Nevada foothills area. Urban aerosols and trace gases experienced significant physical and chemical transformations as they mixed with the reactive biogenic hydrocarbons emitted from the forest. Two heavily-instrumented ground sites – one within the Sacramento urban area and another about 40 km to the northeast in the foothills area – were set up to characterize the evolution of meteorological variables, trace gases, aerosol precursors, aerosol size, composition, and climate related properties in freshly polluted and “aged” urban air. On selected days, the DOE G-1 aircraft was deployed to make similar measurements upwind and across the evolving Sacramento plume in the morning and again in the afternoon. The NASA B-200 aircraft, carrying remote sensing instruments, was also deployed to characterize the vertical and horizontal distribution of aerosols and aerosol optical properties within and around the plume. This overview provides: (a) the scientific background and motivation for the study, (b) the operational and logistical information pertinent to the execution of the study, (c) an overview of key observations and initial findings from the aircraft and ground-based sampling platforms, and (d) a roadmap of planned data analyses and focused modeling efforts that will facilitate the integration of new knowledge into improved representations of key aerosol processes and properties in climate models.

Description

© Author(s) 2012. This work is distributed
under the Creative Commons Attribution 3.0 License.

Published online at: http://dx.doi.org/10.5194/acp-12-7647-2012

DOI
10.5194/acp-12-7647-2012
Persistent Identifier
http://archives.pdx.edu/ds/psu/15196
Citation Information
Zaveri, R. A., Shaw, W. J., Cziczo, D. J., Schmid, B., Ferrare, R. A., Alexander, M. L., Alexandrov, M., Alvarez, R. J., Arnott, W. P., Atkinson, D. B., Baidar, S., Banta, R. M., Barnard, J. C., Beranek, J., Berg, L. K., Brechtel, F., Brewer, W. A., Cahill, J. F., Cairns, B., Cappa, C. D., Chand, D., China, S., Comstock, J. M., Dubey, M. K., Easter, R. C., Erickson, M. H., Fast, J. D., Floerchinger, C., Flowers, B. A., Fortner, E., Gaffney, J. S., Gilles, M. K., Gorkowski, K., Gustafson, W. I., Gyawali, M., Hair, J., Hardesty, R. M., Harworth, J. W., Herndon, S., Hiranuma, N., Hostetler, C., Hubbe, J. M., Jayne, J. T., Jeong, H., Jobson, B. T., Kassianov, E. I., Kleinman, L. I., Kluzek, C., Knighton, B., Kolesar, K. R., Kuang, C., Kubátová, A., Langford, A. O., Laskin, A., Laulainen, N., Marchbanks, R. D., Mazzoleni, C., Mei, F., Moffet, R. C., Nelson, D., Obland, M. D., Oetjen, H., Onasch, T. B., Ortega, I., Ottaviani, M., Pekour, M., Prather, K. A., Radney, J. G., Rogers, R. R., Sandberg, S. P., Sedlacek, A., Senff, C. J., Senum, G., Setyan, A., Shilling, J. E., Shrivastava, M., Song, C., Springston, S. R., Subramanian, R., Suski, K., Tomlinson, J., Volkamer, R., Wallace, H. W., Wang, J., Weickmann, A. M., Worsnop, D. R., Yu, X.-Y., Zelenyuk, A., and Zhang, Q.: Overview of the 2010 Carbonaceous Aerosols and Radiative Effects Study (CARES), Atmos. Chem. Phys., 12, 7647-7687, doi:10.5194/acp-12-7647-2012, 2012.