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Article
Localized singlets and ferromagnetic fluctuations in the dilute magnetic topological insulator Sn0.95Mn0.05Te
Ames Laboratory Accepted Manuscripts
  • David Vaknin, Iowa State University and Ames Laboratory
  • Santanu Pakhira, Ames Laboratory
  • Deborah L. Schlagel, Ames Laboratory
  • Farhan Islam, Iowa State University
  • Jianhua Zhang, Iowa State University
  • D. M. Pajerowski, Oak Ridge National Laboratory
  • Cai-Zhuang Wang, Ames Laboratory
  • David C. Johnston, Iowa State University and Ames Laboratory
  • Robert J. McQueeney, Iowa State University and Ames Laboratory
Publication Date
4-1-2020
Department
Ames Laboratory; Physics and Astronomy
OSTI ID+
1615528
Report Number
IS-J 10210
DOI
10.1103/PhysRevB.101.140406
Journal Title
Physical Review B
Abstract

The development of long-range ferromagnetic (FM) order in dilute magnetic topological insulators can induce dissipationless electronic surface transport via the quantum anomalous Hall effect. We measure the magnetic excitations in a prototypical magnetic topological crystalline insulator, Sn0.95Mn0.05Te, using inelastic neutron scattering. Neutron diffraction and magnetization data indicate that our Sn0.95Mn0.05Te sample has no FM long-range order above a temperature of 2 K. However, we observe slow, collective FM fluctuations (<70μeV), indicating proximity to FM order. We also find a series of sharp peaks originating from local excitations of antiferromagnetically (AF) coupled and isolated Mn-Mn dimers with JAF=460μeV. The simultaneous presence of collective and localized components in the magnetic spectra highlight different roles for substituted Mn ions, with competition between FM order and the formation of AF-coupled Mn-Mn dimers.

DOE Contract Number(s)
AC02-07CH11358
Language
en
Publisher
Iowa State University Digital Repository, Ames IA (United States)
Citation Information
David Vaknin, Santanu Pakhira, Deborah L. Schlagel, Farhan Islam, et al.. "Localized singlets and ferromagnetic fluctuations in the dilute magnetic topological insulator Sn0.95Mn0.05Te" Vol. 101 Iss. 14 (2020) p. 140406(R)
Available at: http://works.bepress.com/d_l_schlagel/144/