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Chiral Light Intrinsically Couples to Extrinsic/Pseudo-Chiral Metasurfaces made of Tilted Gold Nanowires
Scientific Reports
  • Alessandro Belardini, Sapienza Università di Roma
  • Marco Centini, Sapienza Università di Roma
  • Grigore Leahu, Sapienza Università di Roma
  • David C. Hooper, University of Bath
  • Roberto Li Voti, Sapienza Università di Roma
  • Eugenio Fazio, Sapienza Università di Roma
  • Joseph W. Haus, University of Dayton
  • Andrew Sarangan, University of Dayton
  • Ventsislav K. Valev, University of Bath
  • Concita Sibilia, Sapienza Università di Roma
Document Type
Article
Publication Date
8-1-2016
Abstract

Extrinsic or pseudo-chiral (meta)surfaces have an achiral structure, yet they can give rise to circular dichroism when the experiment itself becomes chiral. Although these surfaces are known to yield differences in reflected and transmitted circularly polarized light, the exact mechanism of the interaction has never been directly demonstrated. Here we present a comprehensive linear and nonlinear optical investigation of a metasurface composed of tilted gold nanowires. In the linear regime, we directly demonstrate the selective absorption of circularly polarised light depending on the orientation of the metasurface. In the nonlinear regime, we demonstrate for the first time how second harmonic generation circular dichroism in such extrinsic/pseudo-chiral materials can be understood in terms of effective nonlinear susceptibility tensor elements that switch sign depending on the orientation of the metasurface. By providing fundamental understanding of the chiroptical interactions in achiral metasurfaces, our work opens up new perspectives for the optimisation of their properties.

Inclusive pages
1-9
ISBN/ISSN
2045-2322
Document Version
Published Version
Comments

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This work is licensed under a Creative Commons Attribution 4.0 International License. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/

Publisher
Macmillan Publishers
Peer Reviewed
Yes
Citation Information
Alessandro Belardini, Marco Centini, Grigore Leahu, David C. Hooper, et al.. "Chiral Light Intrinsically Couples to Extrinsic/Pseudo-Chiral Metasurfaces made of Tilted Gold Nanowires" Scientific Reports Vol. 6 (2016)
Available at: http://works.bepress.com/andrew_sarangan/14/